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  • (-) PSI Laboratories = Catalysis and Sustainable Chemistry LSK
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Selective oxidative dehydrogenation of ethane and propane over copper-containing mordenite: insights into reaction mechanism and product protection
Artsiusheuski, M. A., Verel, R., van Bokhoven, J. A., & Sushkevich, V. L. (2023). Selective oxidative dehydrogenation of ethane and propane over copper-containing mordenite: insights into reaction mechanism and product protection. Angewandte Chemie International Edition, 62(44), e202309180 (11 pp.). https://doi.org/10.1002/anie.202309180
Controlling the strong metal-support interaction overlayer structure in Pt/TiO<sub>2</sub> catalysts prevents particle evaporation
Beck, A., Frey, H., Huang, X., Clark, A. H., Goodman, E. D., Cargnello, M., … van Bokhoven, J. A. (2023). Controlling the strong metal-support interaction overlayer structure in Pt/TiO2 catalysts prevents particle evaporation. Angewandte Chemie International Edition, 135(27), e202301468 (7 pp.). https://doi.org/10.1002/anie.202301468
Methane oxidation over Cu<sup>2+</sup>/[CuOH]<sup>+</sup> pairs and site‐specific kinetics in copper mordenite revealed by operando electron paramagnetic resonance and UV‐visible spectroscopy
Fischer, J. W. A., Brenig, A., Klose, D., van Bokhoven, J. A., Sushkevich, V. L., & Jeschke, G. (2023). Methane oxidation over Cu2+/[CuOH]+ pairs and site‐specific kinetics in copper mordenite revealed by operando electron paramagnetic resonance and UV‐visible spectroscopy. Angewandte Chemie International Edition, 62(34), e202303574 (10 pp.). https://doi.org/10.1002/anie.202303574
Dynamical equilibrium between Brønsted and Lewis sites in zeolites: framework‐associated octahedral aluminum
Jin, M., Ravi, M., Lei, C., Heard, C. J., Brivio, F., Tošner, Z., … Nachtigall, P. (2023). Dynamical equilibrium between Brønsted and Lewis sites in zeolites: framework‐associated octahedral aluminum. Angewandte Chemie International Edition, 62(31), e202306183 (6 pp.). https://doi.org/10.1002/anie.202306183
Platinum‐iron(II) oxide sites directly responsible for preferential carbon monoxide oxidation at ambient temperature: an operando X‐ray absorption spectroscopy study
Sadykov, I. I., Sushkevich, V. L., Krumeich, F., Nuguid, R. J. G., van Bokhoven, J. A., Nachtegaal, M., & Safonova, O. (2023). Platinum‐iron(II) oxide sites directly responsible for preferential carbon monoxide oxidation at ambient temperature: an operando X‐ray absorption spectroscopy study. Angewandte Chemie International Edition, 62(1), e202214032 (11 pp.). https://doi.org/10.1002/anie.202214032
Assessing the productivity of the direct conversion of methane‐to‐methanol over copper‐exchanged zeolite omega (MAZ) via oxygen looping
Wieser, J., Knorpp, A. J., Stoian, D. C., Rzepka, P., Newton, M. A., & van Bokhoven, J. A. (2023). Assessing the productivity of the direct conversion of methane‐to‐methanol over copper‐exchanged zeolite omega (MAZ) via oxygen looping. Angewandte Chemie International Edition, 62(40), e202305140 (9 pp.). https://doi.org/10.1002/anie.202305140
Origin of the activity trend in the oxidative dehydrogenation of ethanol over VO<em><sub>x</sub></em>/CeO<sub>2</sub>
Zabilska, A., Zabilskiy, M., Nuguid, R. J. G., Clark, A. H., Sadykov, I. I., Nachtegaal, M., … Safonova, O. V. (2023). Origin of the activity trend in the oxidative dehydrogenation of ethanol over VOx/CeO2. Angewandte Chemie International Edition, 62(18), e202301297 (8 pp.). https://doi.org/10.1002/anie.202301297
Drastic events and gradual change define the structure of an active copper-zinc-alumina catalyst for methanol synthesis
Beck, A., Newton, M. A., Zabilskiy, M., Rzepka, P., Willinger, M. G., & van Bokhoven, J. A. (2022). Drastic events and gradual change define the structure of an active copper-zinc-alumina catalyst for methanol synthesis. Angewandte Chemie International Edition, 61(15), e202200301 (8 pp.). https://doi.org/10.1002/anie.202200301
Electron diffraction enables the mapping of coke in ZSM-5 micropores formed during methanol-to-hydrocarbons conversion
Wennmacher, J. T. C., Mahmoudi, S., Rzepka, P., Lee, S. S., Gruene, T., Paunović, V., & van Bokhoven, J. A. (2022). Electron diffraction enables the mapping of coke in ZSM-5 micropores formed during methanol-to-hydrocarbons conversion. Angewandte Chemie International Edition, 61(29), e202205413 (5 pp.). https://doi.org/10.1002/anie.202205413
Heterogeneously‐catalyzed aerobic oxidation of methane to a methyl derivative
Blankenship, A. N., Ravi, M., Newton, M. A., & van Bokhoven, J. A. (2021). Heterogeneously‐catalyzed aerobic oxidation of methane to a methyl derivative. Angewandte Chemie International Edition, 60(33), 18138-18143. https://doi.org/10.1002/anie.202104153
Spatio‐chemical heterogeneity of defect‐engineered metal‐organic framework crystals revealed by full‐field tomographic X‐ray absorption spectroscopy
Ferreira Sanchez, D., Ihli, J., Zhang, D., Rohrbach, T., Zimmerman, P., Lee, J., … Ranocchiari, M. (2021). Spatio‐chemical heterogeneity of defect‐engineered metal‐organic framework crystals revealed by full‐field tomographic X‐ray absorption spectroscopy. Angewandte Chemie International Edition, 60(18), 10032-10039. https://doi.org/10.1002/anie.202013422
Paired copper monomers in zeolite omega: the active site for methane‐to‐methanol conversion
Knorpp, A. J., Pinar, A. B., Baerlocher, C., McCusker, L. B., Casati, N., Newton, M. A., … van Bokhoven, J. A. (2021). Paired copper monomers in zeolite omega: the active site for methane‐to‐methanol conversion. Angewandte Chemie International Edition, 60(11), 5854-5858. https://doi.org/10.1002/anie.202014030
Methane‐to‐methanol on mononuclear copper(II) sites supported on Al<sub>2</sub>O<sub>3</sub>: structure of active sites from electron paramagnetic resonance
Meyet, J., Ashuiev, A., Noh, G., Newton, M. A., Klose, D., Searles, K., … Copéret, C. (2021). Methane‐to‐methanol on mononuclear copper(II) sites supported on Al2O3: structure of active sites from electron paramagnetic resonance. Angewandte Chemie International Edition, 60(29), 16200-16207. https://doi.org/10.1002/anie.202105307
Direct evidence on the mechanism of methane conversion under non-oxidative conditions over iron-modified silica: the role of propargyl radicals Unveiled
Puente-Urbina, A., Pan, Z., Paunović, V., Šot, P., Hemberger, P., & van Bokhoven, J. A. (2021). Direct evidence on the mechanism of methane conversion under non-oxidative conditions over iron-modified silica: the role of propargyl radicals Unveiled. Angewandte Chemie International Edition, 60(45), 24002-24007. https://doi.org/10.1002/anie.202107553
Identification of kinetic and spectroscopic signatures of copper sites for direct oxidation of methane to methanol
Sushkevich, V. L., Artsiusheuski, M., Klose, D., Jeschke, G., & van Bokhoven, J. A. (2021). Identification of kinetic and spectroscopic signatures of copper sites for direct oxidation of methane to methanol. Angewandte Chemie International Edition, 60(29), 15944-15953. https://doi.org/10.1002/anie.202101628
Mechanistic study of carbon dioxide hydrogenation over Pd/ZnO‐based catalysts: the role of palladium‐zinc alloy in selective methanol synthesis
Zabilskiy, M., Sushkevich, V. L., Newton, M. A., Krumeich, F., Nachtegaal, M., & van Bokhoven, J. A. (2021). Mechanistic study of carbon dioxide hydrogenation over Pd/ZnO‐based catalysts: the role of palladium‐zinc alloy in selective methanol synthesis. Angewandte Chemie International Edition, 60(31), 17053-17059. https://doi.org/10.1002/anie.202103087
Hierarchical structure of NiMo hydrodesulfurization catalysts determined by ptychographic X‐ray computed tomography
Ihli, J., Bloch, L., Krumeich, F., Wakonig, K., Holler, M., Guizar-Sicairos, M., … van Bokhoven, J. A. (2020). Hierarchical structure of NiMo hydrodesulfurization catalysts determined by ptychographic X‐ray computed tomography. Angewandte Chemie International Edition, 59(39), 17266-17271. https://doi.org/10.1002/anie.202008030
Pathways of methane transformation over copper‐exchanged mordenite as revealed by <em>in situ</em> NMR and IR spectroscopy
Sushkevich, V. L., Verel, R., & van Bokhoven, J. A. (2020). Pathways of methane transformation over copper‐exchanged mordenite as revealed by in situ NMR and IR spectroscopy. Angewandte Chemie International Edition, 59(2), 910-918. https://doi.org/10.1002/anie.201912668
Monomeric copper(II) sites supported on alumina selectively convert methane to methanol
Meyet, J., Searles, K., Newton, M. A., Wörle, M., van Bavel, A. P., Horton, A. D., … Copéret, C. (2019). Monomeric copper(II) sites supported on alumina selectively convert methane to methanol. Angewandte Chemie International Edition, 58(29), 9841-9845. https://doi.org/10.1002/anie.201903802
Rapid structure determination of microcrystalline molecular compounds using electron diffraction
Gruene, T., Wennmacher, J. T. C., Zaubitzer, C., Holstein, J. J., Heidler, J., Fecteau-Lefebvre, A., … Pantelic, R. (2018). Rapid structure determination of microcrystalline molecular compounds using electron diffraction. Angewandte Chemie International Edition, 57(50), 16313-16317. https://doi.org/10.1002/anie.201811318